 | Sienna Miller als Tippi Hedren |
 | Toby Jones als Alfred Hitchcock |
 | Imelda Staunton als Alma Reville Hitchcock |
 | Conrad Kemp als Evan Hunter |
 | Penelope Wilton als Peggy Robertson |
 | Angelina Ingpen als Melanie |
| Candice D'Arcy als Josephine Milton |
 | Carl Beukes als Jim Brown |
| Kate Tilley als Rita Riggs |
 | Aubrey Shelton als Maitre D |
 | Leon Clingman als Ray Berwick |
 | Patrick Lyster als Bob Boyle |
| Adrian Galley als Martin Balsam (uncredited) |
| Louis Joubert als Reporter (uncredited) |
| Leon Kowalski als Photographer (uncredited) |
 | Sean Cameron Michael als Robert Burks (uncredited) |
 | Carel Nel als Clapper Loader (uncredited) |
| Julian Jarrold | Director |
| Gwyneth Hughes | Writer |
| Philip Miller | Original Music Composer |
| Andrew Hulme | Editor |
| Amanda Jenks | Producer |
| John Pardue | Director of Photography |
| Darryl Hammer | Production Design |
| Christa Schamberger | Casting |
| Mito Skellern | Casting |
| Gail Stevens | Casting |
| Genevieve Hofmeyr | Co-Producer |
| Marvin Saven | Co-Producer |
| Christian Assange | Co-Producer |
| Lucy Richer | Executive Producer |
| Leanne Klein | Executive Producer |
| Dianne Beatty | Line Producer |
| Aparna Jayachandran | Script Supervisor |
| Diana Cilliers | Costume Design |
| Donald Spoto | Book |
| Alex Graham | Executive Producer |
| Di Sole | Art Direction |
| Ashleigh Tobias | Set Decoration |
| Daleen Badenhorst | Prosthetic Makeup Artist |
| Neill Gorton | Prosthetic Designer |
| Chris Lyons | Special Effects Makeup Artist |
| Rob Mayor | Prosthetics |
| Nadine Prigge | Makeup & Hair |
| Clinton Smith | Prosthetic Makeup Artist |
| Francesca Van Der Feyst | Key Hair Stylist |
